Experimental and Kinetic Modeling Study of Cyclohexane and Its Mono-alkylated Derivatives Combustion

Nonfiction, Science & Nature, Science, Physics, Thermodynamics, Biological Sciences, Environmental Science, Technology
Cover of the book Experimental and Kinetic Modeling Study of Cyclohexane and Its Mono-alkylated Derivatives Combustion by Zhandong Wang, Springer Singapore
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Author: Zhandong Wang ISBN: 9789811056932
Publisher: Springer Singapore Publication: January 23, 2018
Imprint: Springer Language: English
Author: Zhandong Wang
ISBN: 9789811056932
Publisher: Springer Singapore
Publication: January 23, 2018
Imprint: Springer
Language: English

This thesis investigates the combustion chemistry of cyclohexane, methylcyclohexane, and ethylcyclohexane on the basis of state-of-the-art synchrotron radiation photoionization mass spectrometry experiments, quantum chemistry calculations, and extensive kinetic modeling. It explores the initial decomposition mechanism and distribution of the intermediates, proposes a novel formation mechanism of aromatics, and develops a detailed kinetic model to predict the three cycloalkanes’ combustion properties under a wide range of conditions. Accordingly, the thesis provides an essential basis for studying much more complex cycloalkanes in transport fuels and has applications in engine and fuel design, as well as emission control.

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This thesis investigates the combustion chemistry of cyclohexane, methylcyclohexane, and ethylcyclohexane on the basis of state-of-the-art synchrotron radiation photoionization mass spectrometry experiments, quantum chemistry calculations, and extensive kinetic modeling. It explores the initial decomposition mechanism and distribution of the intermediates, proposes a novel formation mechanism of aromatics, and develops a detailed kinetic model to predict the three cycloalkanes’ combustion properties under a wide range of conditions. Accordingly, the thesis provides an essential basis for studying much more complex cycloalkanes in transport fuels and has applications in engine and fuel design, as well as emission control.

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