Design, Synthesis and Characterization of new Supramolecular Architectures

Nonfiction, Science & Nature, Technology, Nanotechnology, Science, Chemistry, Physical & Theoretical
Cover of the book Design, Synthesis and Characterization of new Supramolecular Architectures by Massimo Baroncini, Springer Berlin Heidelberg
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Author: Massimo Baroncini ISBN: 9783642192852
Publisher: Springer Berlin Heidelberg Publication: April 15, 2011
Imprint: Springer Language: English
Author: Massimo Baroncini
ISBN: 9783642192852
Publisher: Springer Berlin Heidelberg
Publication: April 15, 2011
Imprint: Springer
Language: English

This thesis focuses on the bottom-up design, construction and operation of supramolecular systems capable of behaving as devices and machines on the molecular scale, which is a topic of great interest in nanoscience and a fascinating challenge in nanotechnology. In particular, the systems investigated here include: polyviologen dendrimers capable of behaving as hosts and chargestoring devices; molecular machines based on pseudorotaxanes/rotaxanes and operated by photoinduced proton transfer, or photoisomerization reactions; and a simple unimolecular multiplexer/demultiplexer. The systems have been characterized using a variety of techniques including absorption and emission spectra, laser flash photolysis, NMR spectroscopy, electrochemical experiments, stopped flow measurements. This research addresses a large number of open problems in the nanosciences, dealing with a wide range of the most advanced applications of supramolecular systems.

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This thesis focuses on the bottom-up design, construction and operation of supramolecular systems capable of behaving as devices and machines on the molecular scale, which is a topic of great interest in nanoscience and a fascinating challenge in nanotechnology. In particular, the systems investigated here include: polyviologen dendrimers capable of behaving as hosts and chargestoring devices; molecular machines based on pseudorotaxanes/rotaxanes and operated by photoinduced proton transfer, or photoisomerization reactions; and a simple unimolecular multiplexer/demultiplexer. The systems have been characterized using a variety of techniques including absorption and emission spectra, laser flash photolysis, NMR spectroscopy, electrochemical experiments, stopped flow measurements. This research addresses a large number of open problems in the nanosciences, dealing with a wide range of the most advanced applications of supramolecular systems.

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